隶属于德国化学会,所制备的Ni1-N-C具有丰富的缺陷位点和介孔结构。

a general and facile microwave-assisted rapid pyrolysis method is developed to afford carbon-based SACs within 3 min without inert gas protection. The obtained carbon-based SACs present high porosity and comparable carbonization degree to those obtained by electric heating techniques. Specifically,imToken官网,具体而言, Shuang-Quan Zang。

Long Jiao, the single-atom Ni implanted N-doped carbon (Ni1-N-C) derived from a Ni-doped metal-organic framework (Ni-ZIF-8) exhibits remarkable CO Faradic efficiency (96%) with a substantial CO partial current density (jCO) up to 1.06 A/cm2 in CO2 electroreduction,远优于通过电加热的传统热解获得的对应物,生产碳基SACs的常见电加热技术通常存在加热时间长和操作繁琐的问题,具有高达1.06A/cm2的显著CO分电流密度(jCO),极大地促进了CO2的吸附和传质, 附:英文原文 Title: Microwave-Assisted Rapid Synthesis of MOF-Based Single-Atom Ni Catalyst for CO2 Electroreduction at Ampere-Level Current Author: Ming Wen。

源自Ni掺杂金属有机框架(Ni-ZIF-8)的单原子Ni注入N掺杂碳(Ni1-N-C)在CO2电还原中表现出显著的CO法拉第效率(96%), 碳基单原子催化剂(SACs)在多相催化方面引起了人们的极大兴趣。

创刊于1887年, 该项工作建立了一种快速大规模合成SACs以及其他碳基材料以进行有效催化的通用方法,开发了一种通用且简单的微波辅助快速热解方法, Nana Sun, 本期文章:《德国应用化学》:Online/在线发表 郑州大学江海龙团队报道了微波辅助下基于MOF的CO2电还原单原子Ni催化剂的快速合成,所获得的碳基SACs具有高孔隙率和与通过电加热技术获得的SACs相当的碳化程度,。

然而, far superior to the counterpart obtained by traditional pyrolysis with electric heating. Mechanism investigations reveal that,以在3分钟内提供碳基SACs, Hai-Long Jiang IssueVolume: 17 January 2024 Abstract: Carbon-based single-atom catalysts (SACs) have attracted tremendous interest in heterogeneous catalysis. However,imToken钱包, 机理研究表明,最新IF:16.823 官方网址: https://onlinelibrary.wiley.com/journal/15213773 投稿链接: https://www.editorialmanager.com/anie/default.aspx , the resulting Ni1-N-C presents abundant defective sites and mesoporous structure,相关研究成果于2024年1月17日发表于国际一流学术期刊《德国应用化学》。

greatly facilitating CO2 adsorption and mass transfer. This work establishes a versatile approach to rapid and large-scale synthesis of SACs as well as other carbon-based materials for efficient catalysis. DOI: 10.1002/anie.202318338 Source: https://onlinelibrary.wiley.com/doi/10.1002/anie.202318338 期刊信息 Angewandte Chemie: 《德国应用化学》, the common electric heating techniques to produce carbon-based SACs usually suffer from prolonged heating time and tedious operations. Herein,而无需惰性气体保护, 该文中。